A partnership of academic & research institutions, HathiTrust is a collection of digitized titles from libraries around the world, including many older publications from federal and state agencies.
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Contains statistical trends of elementary, secondary, and higher education. Covers 1850-1990, but years vary among datasets. Also includes a useful overview of the history of educational statistics and how they've changed over the years.
Provides easy access to US demographic data, and allows you to create maps and reports. Education data goes back to 1850.
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U.S. Dept. of Education Publications
The National Center for Education Statistics provides data primarily from the early 2000s to present. Earlier publications may have been digitized by libraries participating in HathiTrust. Examples include